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In schematics and cartoons, the gas-liquid interface is often drawn as solid lines that aid in distinguishing the separation of the two phases. However, on the molecular level, the structure, shape, and size of the gas-liquid interface remain elusive. Furthermore, the interactions of molecules at gas-liquid interfaces must be considered in various contexts, including atmospheric chemical reactions, wettability of surfaces, and numerous other relevant phenomena. Hence, understanding the structure and interactions of molecules at the gas