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Efficiencies of artificial photosynthetic and photocatalytic systems depend on their ability to generate long-lived charge-separated (CS) states in photoinduced electron transfer (PET) reactions. PET, in most cases, is followed by an ultrafast back electron transfer, which severely reduces lifetime and quantum yield of CS states. Generation of a long-lived CS state is an important goal in the study of PET reactions. Herein, we report that this goal is achieved using a hierarchically self-assembled anthracene-methyl viologen donor-accepto
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