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This finding proposes the complex magnetic properties in the layered cobalt oxides with multiple magnetic sublattices in the coexistence system of itinerant and localized electrons.We report on the isolation of a new family of μ-carboxylato-bridged metallocrown (MC) compounds by self-assembly of the recently isolated hexadentate tris(2-pyridylmethyl)amine ligand tpada2- incorporating two carboxylate units with metal cations. Twelve-membered MCs of manganese of the type 12-MC-3, namely, [MnII(tpada)3(M)(H2O)n]2+ (Mn3M) (M = Mn2+ (n =
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