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65) whereas amorphous arrangements can be observed in layers with either low (down to ∼0.53) or high (∼0.65) volume fraction. Lastly, we demonstrate via targeted additional experiments and SAXS measurements, that the packing structure of the layers is mainly driven by the formation of aggregates and their subsequent packing, and not by the competition between Brownian diffusion and convection. This highlights that a second dimensionless ratio in addition to the Peclet number should be taken into account, namely the agg