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The Fourier-transform infrared spectrometry (FTIR), and X-ray photoelectron spectroscopy (XPS) results implied that the adsorption process followed via the electrostatic interactions, hydrogen bonding, and π-π stacking between the functionality of hydrogel and aromatic rings of DFS. Considering the low-cost, and an excellent DFS removal capacity, the natural composite ALB/PEI hydrogel could be a promising adsorbent for the treatment of DFS contaminated wastewater. Nanoparticles are recently employed as a new strategy to directly kill pat