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Bilayer spin crossover (SCO)@polymer nanocomposites show robust and controllable actuation cycles upon an electrical stimulus. The anisotropic shape of the embedded particles as well as the mechanical coupling between the SCO particles and the matrix can substantially intensify the work output of the actuators.In this short review, we provide an overview of our efforts in developing a family of anodically coloring electrochromic (EC) molecules that are fully transparent and colorless in the charge neutral state, and that can rapidly swit