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Owing to their unique superiorities in chemical and photoluminescence (PL) stability, low toxicity, biocompatibility, and easy functionalization, graphene quantum dots (GQDs) are widely used in cell imaging, probes, and sensors. However, further development and deeper research of GQDs are restricted by their imprecise and complex structure and accompanying controversial PL mechanism. In this work, two kinds of structure-defined water-soluble GQDs, with different oxidation degrees, are synthesized from molecules using bottom-up synthese
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