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The electronic coupling matrix element HAB is an essential ingredient of most electron-transfer theories. HAB depends on the overlap between donor and acceptor wave functions and is affected by the involved states' spin. We classify the spin-state effects into three categories orbital occupation, spin-dependent electron density, and density delocalization. The orbital occupancy reflects the diverse chemical nature and reactivity of the spin states of interest. The effect of spin-dependent density is related to a more compact electron de

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