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Finally, we lay out some general ideas for how the knowledge gained could ultimately lead to new design principles for tuning molecular excitation energies as well as for diagnosing possible shortcomings of commonly used electronic structure methods.A diversified and biocompatible rhythmic deformation (RD) system is successfully fabricated by coupling a heterogeneous hydrogel with a pH oscillator. By tailoring the geometry of the building blocks, a heterogeneous hydrogel actuator with diversity could be easily constructed through inter