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The shell thickness was tuned from 9.8 to 29.5 nm by simply varying the silver-ion concentration. A key factor was the amount of added PEI because excess PEI would result in the formation of silver nanoparticles in the bulk solution phase, while too little PEI would produce incomplete shells. The optimum mass ratio of PEI-to-silica particles was determined to be 1.0 for the experimental conditions in this study. The mixing sequence of the reaction solutions was also important because PEI had to be mixed with silica particles first to ens
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