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This strategy of grafting CNTs at a high-density opens a new avenue for the interfacial regulation of structural composites, ultra-capacitor, sensor, and catalytic materials.Marine biofouling is a ubiquitous and longstanding challenge that causes both economic and environmental problems. To address this, several antifouling strategies have been proposed, such as the release of biocidal compounds or surface chemical/physical design. Here we report a coating with surface structures (chemical heterogeneity) triggered by phase segregation, w