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We believe that the PLAL process proposed in this study will serve as a simple and one-step route for designing S-GQDs and opens up to opportunities for their potential applications.Structured beams, conventionally generated through the spatial mode conversion of the Gaussian laser beams, have attracted great interest in recent years. Optical parametric oscillators (OPOs) have demonstrated the potential for the generation of tunable structured beams directly from an input pump source. However, to date, a particular OPO design has been s