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In this work, the heteroatoms (Zn + C) and cyano (CN) group co-decorated permeable g-C3N4 nanosheets (DCNNS) photocatalysts were successfully synthesized through direct calcination associated with combined urea and metal-organic frameworks. The enhanced DCNNS displayed a maximum H2 evolution rate of ~484.09 μmol/h with a quantum efficiency of ~3.43% at 420 nm, as well as the photocatalytic U(VI) reduction task ended up being improved by ~6.09 times. The improved photocatalytic overall pe