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The discovery of the considered compounds involved substantial theoretical contributions. We address future challenges facing the design of materials at high pressure and provide perspectives on research directions with significant potential for future discoveries.Janus two-dimensional materials (2DMs) are a novel class of 2DMs in which the two faces of the material are either asymmetrically functionalized or are exposed to a different local environment. The diversity of the properties imparted to the two opposing sides enables the desig
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