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In the process of VO2 hydrogenation, the electron transfer only occurs between hydrogen and its connected oxygen atoms on the VO2 surface, and vanadium atoms just play an intermediary role.We herein report a series of near-linear trinuclear complexes [Co2Ln(HL)4(NO3)](NO3)2 (where HL = (2-methoxy-6-[(E)-2'-hydroxymethyl-phenyliminomethyl]-phenolate) with Ln(III) = La (1), Ce (2), Pr (3)). For the comparative study, we have also included the recently reported analogous complexes of Gd(III), Tb(III), and Dy(III) (complexes 4-6) with the s
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