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Liquid crystalline cellulose nanocrystals (CNCs) which can change their structural and optical properties in an electric field could be a new choice for advanced optoelectronic devices. Unfortunately, the exploration of its performance in an electric field is underdeveloped. Hence, we reveal some interesting dielectric coupling activities of liquid crystalline CNC in an electric field. The CNC tactoid is shown to orient its helix axis normal to the electric field direction. Then, as a function of the electric field strength and frequen