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The data described in this paper were collected in two watersheds - Azuga-suba watershed in Angacha woreda (district) of Southern Nations, Nationalities and Peoples (SNNP) region and Yesir watershed of Bure woreda (district) of the Amhara region - in Ethiopia. The data were collected from 379 households with the main objective being to assess the factors constraining the adoption of sustainable land management technologies (SLMT) that enhance soil organic carbon sequestration. The data were collected using a structured questionnaire t