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Comprehensive observations have been carried out in Beijing to investigate the impact of the Clean Air Action implemented in 2013 on changes in aerosol chemistry characteristics in heating seasons of 2016-2017 and 2017-2018. Results showed that PM2.5, SO2, NO2, NH3, O3 and CO concentrations decreased by 40.9%, 46.0%, 29.0%, 40.6%, 11.0% and 44.4%, respectively. Significant decreases were also observed for NO3- (32.5%), SO42- (52.9%), NH4+ (56.0%), Cl- (64.6%) and K+ (68.2%), on average. Enhanced PM2.5 pollution has changed from sulfate-d