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19 to 0.11 after 4 min MS. In addition, the MPS results demonstrated the third harmonic amplitude normalized to the iron amount [Formula see text] and harmonic ratio [Formula see text] of signal increase from 8.38 to 10.59 Am kg (Fe) and 24.21-26.60, respectively. Furthermore, the MPI images of the samples after separation showed higher MPI resolution. Therefore, LGMS can be considered as a valuable method to narrow and control the size distribution of MNP for MPI. Therefore, LGMS can be considered as a valuable method to narrow and con