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This study demonstrates the formation of biocompatible magnetic particles into organized structures upon the application of an external magnetic field. The capability to create the structures was examined in silicone-oil suspensions and in a gelatine solution, which is commonly used as a blood plasma expander. Firstly, the carbonyl iron particles were successfully coated with gelatine, mixed with a liquid medium in order to form a magnetorheological suspension, and subsequently the possibility of controlling their rheological parameters