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From these results, we show that machine learning, particularly deep neural networks, can be employed as cost-effective statistical approaches for designing electromagnetic fields to enable desired transitions in these quantum dynamical systems.Molecule like silver quantum clusters ([Agm]n+ QCs) exhibit an ultrasmall size confinement resulting in efficient broadband fluorescence. However, free [Agm]n+ QCs are also chemically active, so their stabilization is required for practical applications. We report in this work a phosphate oxyfluorid