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Morphology-control synthesis is an effective means to tailor surface structure of noble-metal nanocrystals, which offers a sensitive knob for tuning their electrocatalytic properties. The functional molecules are often indispensable in the morphology-control synthesis through preferential adsorption on specific crystal facets, or controlling certain crystal growth directions. In this review, the recent progress in morphology-control synthesis of noble-metal nanocrystals assisted by amino-based functional molecules for electrocatalytic a