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The construction of efficient and superior adsorbed materials for the precise removal of hazardous contaminants from water have gained significant attention by the scientific community. In this work, a facile bimetallic zeolitic-imidazolate framework (CoxZny-JUC-16 by using self-adjusted strategy (SAS) was developed to synthesize various N-doped Co-based hierarchical porous carbon composites through sacrificial template route. A series of highly porous magnetic materials with well-dispersed or reduced Co particle size have been fabrica