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In-depth research on energy storage and conversion is urgently needed; thus, water splitting has become a possible method to achieve sustainable energy utilization. However, traditional carbon material with high graphitization degree exhibits a relatively low electrocatalytic oxygen evolution reaction (OER) and hydrogen evolution reaction (HER) activity as it is electrochemically inert. In this work, according to the Lewis theory of acids and bases and the density functional theory (DFT) results, which show that the enriched heteroatom
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