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Fractals are of fundamental importance in science and technology. Theoretical simulations indicate that Sierpiński triangles (STs) possess specific optical and electronic properties. To study their properties and uncover their potential applications, it is necessary to pack STs into large-scale two-dimensional crystalline structures. Here, a series of ordered structures consisting of ST units are successfully constructed on gold surfaces through coordination between 1,3-bis(4-pyridyl) benzene molecules and Fe atoms. Crystals of STs are
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