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Water contamination due to heavy metal-based toxic oxo-anions (such as CrO42- and TcO4-) is a critical environmental concern that demands immediate mitigation. Herein, we present an effort to counter this issue by a novel chemically stable cationic metal-organic framework (iMOF-2C) with strategic utilization of a ligand with hydrophobic core, known to facilitate such oxo-anion capture process. Moreover, the compound exhibited very fast sieving kinetics for such oxo-anions and a very high uptake capacity for CrO42- (476.3 mg g-1) and Re
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