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Infrared photodissociation spectra of the D2-tagged microhydrated sulfate dianions with three to eight water molecules are presented over a broad spectral range that covers the OH stretching and H2O bending modes of the solvent molecules at higher energies, the sulfate stretching modes of the solute at intermediate energies and the intermolecular solute librational modes at the lowest energies. A low ion temperature combined with messenger-tagging ensures well-resolved vibrational spectra that allow for structure assignments based on a
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