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These modulated approaches and challenges are also instructive for constructing other high-activity energy-related electrocatalysts. © 2020 WILEY-VCH Verlag GmbH Co. KGaA, Weinheim.Recently, 2D transition metal dichalcogenides (TMDs) have become intriguing materials in the versatile field of photonics and optoelectronics because of their strong light-matter interaction that stems from the atomic layer thickness, broadband optical response, controllable optoelectronic properties, and high nonlinearity, as well as compatibility. Nev