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Even though there has been a lot of studies on the magnetic properties of FexTiS2 and their corresponding atomic structures at different Fe concentrations, the dependency of the properties on the Fe atomic arrangement has not been fully clarified yet. In this study, FexTiS2 structures, synthesized by chemical vapor transport technique at Fe concentrations of 0.05, 0.10, 0.15, 0.20 0.25 and 0.33, were observed three-dimensionally using a transmission electron microscope and their corresponding magnetization values were measured using a sup