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© 2020 The Authors.Controlled deposition of colloidal nanoparticles using self-assembly is a promising technique for, for example, manufacturing of miniaturized electronics, and it bridges the gap between top-down and bottom-up methods. However, selecting materials and geometry of the target surface for optimal deposition results presents a significant challenge. Here, we describe a predictive framework based on the Derjaguin-Landau-Verwey-Overbeek theory that allows rational design of colloidal nanoparticle deposition setups. The frame