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In this work, we have designed a magnetoluminescent nanocomposite as a single platform for optical imaging and safe magnetic hyperthermia therapy by optimizing the composition of magnetic nanoparticles and controlling the conjugation strategy of the luminescent lanthanide complex. We have synthesized Co x Mn1-xFe2O4 nanoferrites, with x = 0 to 1 in 0.25 steps, from soft (MnFe2O4) to hard (CoFe2O4) ferrites of size (∼20 nm) following a one-pot oxidative hydrolysis method. We have performed the induction heating study with an aqueous disp