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This work should guide the design of HEA-NPs to expand their potential applications in mechanical structures, medicine, catalysis, and energy storage/conversion.This paper describes a correlation between charge extraction and energy-level alignment at the interface of polymeric hole transport layers and perovskite active layers. By tailoring the composition of the conjugated backbone of the hole transport material, energy levels between perovskites and hole transport layers are varied. Matching the band alignment at perovskite/hole trans