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© The Author(s) (202. Published by Oxford University Press. All rights reserved. For Permissions, please email journals.permissions@oup.com.Exploring oxygen electrodes with superior bifunctional catalytic activity and suitable architecture is an effective strategy to improve the performance of lithium-oxygen (Li-O2) batteries. Herein, the internal electronic structure of Ni2P is regulated by heteroatom Co doping to improve its catalytic activity for oxygen redox reactions. Meanwhile, magnetron sputtering N-doped carbon cloth (N-CC) is
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