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This work contributes to the understanding of the specific interaction between alkali metals and SO2 on deNOx catalysts and provides a novel strategy for the adaptive use of one poisoning substance to counter another for practical NOx reduction.Under solvothermal conditions, a three-dimensional mononuclear crystal AQNU-1, [CH2L)(DPD)(H2O)2]·2DMAn (H2L = 5-(bis(4-carboxybenzyl)amino)isophthalic acid, DPD = 4,4'-(2,5-diethoxy-1,4-phenylene)dipyridine) has been synthesized. The transformations of AQNU-1 to binuclear [Co2(L)(DPD)1.5(H2O)3]·
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