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Slot-die printing, a large-scale deposition technique, is applied to fabricate mesoporous titania films. Printing is interesting, for example, for scaling up solar cells where titania films with an interconnected mesoporous network and a large surface-to-volume ratio are desired as photoanodes. A fundamental understanding of the structure evolution during printing is of high significance in tailoring these films. In this work, we provide important insights into the self-assembly of the slot-die-printed titania/polystyrene-block-poly(et
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