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The present approach provides a basis for understanding the origin of the KR2 CD spectrum and is useful for analyzing the mechanism of chromophore-chromophore interactions in biological systems.Kinetics of photoinduced intramolecular charge separation (CS) and the ensuing ultrafast charge recombination (CR) in electron-donor-acceptor dyads are studied numerically, taking into account the excitation of charge-transfer active intramolecular vibrations and multiple relaxation time scales of the surrounding polar solvent. Both energetic and

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